Category: antimatter

Rydberg Positronium and Stark broadening

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We have recently produced Rydberg positronium atoms in a two step excitation process, using 243 nm light from our broad band pulsed dye laser to excite 2P states, as in our previous Ps spectroscopy measurements. Then, instead of photoionizing with 532 nm light, we used ~ 750 nm light to excite 2p-nd transitions. This process is shown in the energy level diagram below, you can also see a photograph of the green light produced by our Nd:YAG laser pumping the infra red laser.

greenlight

Rydberg

Once the Ps atoms have been excited to a Rydberg state, their lifetime is greatly increased, and they only annihilate once they collide with the vacuum chamber. This leads to a reduced delayed fraction in our positronium SSPALS signal, since there are less gamma ray events occurring on our delayed detection time (to read more about how we detect Ps, read here). This can be seen in our data below where we excited Ps atoms to n = 11.

Rydberg1kv2kv3kv

When atoms are subjected to a high electric field different states are separated and shifted leading to an overall broadening of the spectral line, this effect is known as Stark broadening,  the mixing and shifting of the states is proportional to the strength of the electric field being applied. We are able to observe this effect by varying the voltage  applied to our porous silica target from which Ps atoms are produced, and therefore changing the electric field that the Ps atoms are subjected to. As the voltage is increased, the broadening grows with the eclectic field, thus producing a signal over a wider range of infra red wavelengths, this is shown in the figure above where we plot the delayed fraction over a range of 5.6 nm, changing the voltage applied to our target from from 1 kV to 2 kV and 3 kV.

Positronium formation detected using annihilation radiation energy spectroscopy

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When a positron and an electron annihilate directly, instead of forming a Ps atom, all of their energy is converted into two gamma ray photons, each with 511 keV (the rest mass energy of the electron/positron). However, if an electron and a positron form a Ps atom the annihilation can occur either into two or three photons, depending on the spin state of the Ps atom. The longer-lived Ps state is called ortho-positronium (o-Ps), and in this system the electron and positron spins point in the same direction, so the total spin of the atom is 1. This means that o-Ps has to decay into an odd number of gamma rays in order to conserve angular momentum. Usually this means three photons, as single photon decay can only happen if there is a third body present (this has been observed). The three photon energies are spread out over a large range (but they always add up to 2 x 511 keV). The short-lived Ps state is called para-positronium (p-Ps) and this usually decays into two photons. It is possible for a three photon state to have zero angular momentum, so singlet decay into three photons is not ruled out by momentum considerations, but this mode is suppressed and to a good approximation p-Ps decays into two gamma rays with well-defined energies (i.e., 511 keV). This means that p-Ps decays look very similar to direct electron-positron decays. It also means that we can detect the presence of o-Ps by looking at the energy spectrum of annihilation radiation, as is shown in the graph below.

peakvalley3kV

We are able to measure gamma ray energies using a detector; in this case NaI(TI), or thallium doped sodium iodide. The data shown above were taken with a positron beam fired into a piece of untreated metal, from which we expect hardly any Ps to be made, and also in a silica film, which we know converts about 30% of the incident positrons into the Ps atoms. When the beam hits the metal many events at energies close to 511 keV are detected, since most positrons will annihilate directly into two 511 keV photons.
The production of Ps can be seen when we compare the two curves (red and black lines) shown in the figure. These spectra are normalised to have the same total area, so the excess of counts in the valley region (i.e., energies between about 300 and 500 keV), and the reduction of counts in the photopeak (at 511 keV) is exactly what you would expect if you made positronium: the decay into three photons means there are more photons with energies less than 511 keV.

Ps Spectroscopy

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We have used our ultraviolet laser (a pulsed dye laser), in addition to a green laser, to ionize a significant fraction of the positronium (Ps) atoms produced by our beamline (read here for more details).

We first tune the UV laser to a wavelength of 243 nm, for which the photons have the same energy as the interval between the ground state and the first excited state of the positronium atom.

We carefully time the laser pulse to pass through the cloud of Ps atoms shortly after they’re created, and so many of the atoms absorb the light and become resonantly excited.  The photons in the green laser have sufficient energy to then ionise these excited atoms – separating the positron and electron.  This technique is known as resonant ionisation spectroscopy (RIS).

The positrons are very likely to fall back into the target and annihilate shortly after ionisation occurs, causing more gamma rays to be detected during the prompt peak of our SSPALS traces; with fewer o-Ps annihilations subsequently detected at later times.  An example SSPALS trace, with and without the laser, is shown below.

trace1

We quantify the ionisation by measuring the fraction of delayed annihilations in our SSPALS traces,

f = ∫(B→C)/∫(A→C)

and comparing it to a background measurement without the laser:

S = (flaser on – flaser off)/flaser off

The figure below shows how this ionization signal, S, varies as we tune the UV laser across the resonant wavelength, 243nm, for the 1S-2P transition.

Ps_243nm

The width of the roughly Gaussian line-shape is caused by Doppler broadening, where the atoms moving towards, or away from the laser see a slightly shorter, or longer, wavelength.

The different coloured points represent different voltages applied to the Ps converter. This voltage creates an electric field that attracts and accelerates the positrons, implanting them into the material.  The highest target bias has the narrowest RIS line-shape as the Ps atoms form deep inside the sample and therefore experience more collisions as they make their way back to the surface, which slows them down and reduces the Doppler effect.

Positronium production

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We have made positronium atoms by accelerating positrons from our trap into a porous silica target (which was supplied by Laszlo Liskay in Saclay). We observe the positronium atoms by single shot positronium annihilation lifetime spectroscopy (SSPALS – see here for more information). In this technique we record the gamma photons emitted as the positrons and positronium atoms annihilate. Approximately 50% of the positrons annihilate in the target, producing the large gamma peak observed within the first 20 ns of the trace below. Of the Ps atoms formed, around one quarter are in the very short-lived singlet state (para-positronium). With a lifetime against annihilation of only 120 ps, these atoms also contribute to the large peak. The remaining atoms occupy the triplet state (ortho-positronium) which, with a lifetime against annihilation of 142 ns, lives for over 1000 times longer than p-Ps. This increased lifetime leads to a long tail in the SSPALS trace which is characteristic of positronium generation.

The figure below shows two SSPALS data-sets: one taken with a porous silica target and one with a metal target. In both cases the implantation energy was 1 keV. In the case of the metal target (grey data) we observe no Ps formation, and there is only signal from positron annihilation. However, with  porous silica target (blue data) we record increased signal at times greater than 40 ns after implantation: the signature of Ps formation.

sspals

The porous silica target used in this experiment is an efficient source of cold Ps atoms. The incident positrons are accelerated into the bulk material, where they can either anniliate or form Ps. Once Ps has been formed it can diffuse out of the bulk and into the pores. Collisions with the walls of these pores cools the Ps atoms, ultimately to the lowest quantum state of the potential well. The cooled atoms can then diffuse out of the target through the interconnected pores and into the vacuum.

Ps_drawing

Trapped positrons

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We have trapped positrons, and slowed and cooled them by collisions with N_2 buffer gas and CF_4 cooling gas. The images are 3D plots of the positrons detected on a phosphor screen (see banner at the top of the page).

densityPlots

The left-hand image shows the image resulting from the positron beams impinging on the phosphor screen, passing directly through the trap. The trap shows the distribution with a dip in the centre (see this post for an explanation of where this comes from). The right-hand image was generated by accumulating and cooling positrons in the trap for 1 second. The cloud of trapped positrons is then bunched and accelerated out of the trap and onto the screen.

Next step: we will accelerate these positrons onto a porous target and make positronium!

Positron beam

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We have built a dc beam of positrons. After moderation in solid neon the positrons are magnetically guided away from the source,  through what will be our buffer gas trap, and onto a phosphor screen, located in front of a CCD camera.

Below is a typical image we have recorded of our positron beam.

positrons12May14

The beam has a roughly doughnut-shape, which is determined by the shape of the neon moderator (the moderator has a hollow centre, and so there are fewer of the slow positrons that we detect in the centre of the beam). This beam structure is highlighted in the following figure which shows the recorded beam intensity along a line (shown in the above figure).

positrons12May14

In this experiment we are recording around 2 million positrons per second, several metres downstream of the source.

This is an important step forward in our experiment. The next step will be to accumulate positrons in our trap, and then accelerate them onto a target for Ps production.